| 题名 | Pressure-driven switching of magnetism in layered CrCl3 |
| 作者 | |
| 通讯作者 | Liang,Yongcheng; Wang，Shanmin |
| 发表日期 | 2020-11-26
|
| DOI | |
| 发表期刊 | |
| ISSN | 2040-3364
|
| EISSN | 2040-3372
|
| 卷号 | 12期号:45页码:22935-22944 |
| 摘要 | Layered transition-metal compounds with controllable magnetic behaviors provide many fascinating opportunities for the fabrication of high-performance magneto-electric and spintronic devices. The tuning of their electronic and magnetic properties is usually limited to the change of layer thickness, electrostatic doping, and the control of electric and magnetic fields. However, pressure has been rarely exploited as a control parameter for tailoring their magneto-electric properties. Here, we report a unique pressure-driven isostructural phase transition in layered CrCl3 accompanied by a simultaneous switching of magnetism from a ferromagnetic to an antiferromagnetic ordering. Our experiments, in combination with ab initio calculations, demonstrate that such a magnetic transition hinders the bandgap collapse under pressure, leading to an anomalous semiconductor-to-semiconductor transition. Our findings not only reveal the potential applications of this material in electronic and spintronic devices but also establish the basis for exploring unusual phase transitions in layered transition-metal compounds. |
| 相关链接 | [Scopus记录] |
| 收录类别 | |
| 语种 | 英语
|
| 学校署名 | 第一
; 通讯
|
| 资助项目 | Guangdong Innovative & Entrepreneurial Research Team Program[2016ZT06C279]
; Key Research Platforms and Research Projects of Universities in Guangdong Province[2018KZDXM062]
; National Natural Science Foundation of China[51671126][11027405]
; Science Challenging Program[JCKY2016212A501]
; Shenzhen Peacock Plan[KQTD2016053019134356]
|
| WOS研究方向 | Chemistry
; Science & Technology - Other Topics
; Materials Science
; Physics
|
| WOS类目 | Chemistry, Multidisciplinary
; Nanoscience & Nanotechnology
; Materials Science, Multidisciplinary
; Physics, Applied
|
| WOS记录号 | WOS:000593021300006
|
| 出版者 | |
| EI入藏号 | 20205009598107
|
| EI主题词 | Chlorine compounds
; Calculations
; Antiferromagnetism
; Chromium compounds
; Semiconductor doping
|
| EI分类号 | Metallurgy and Metallography:531
; Magnetism: Basic Concepts and Phenomena:701.2
; Semiconducting Materials:712.1
; Mathematics:921
|
| Scopus记录号 | 2-s2.0-85096888708
|
| 来源库 | Scopus
|
| 引用统计 |
被引频次[WOS]：19
|
| 成果类型 | 期刊论文 |
| 条目标识符 | http://sustech.caswiz.com/handle/2SGJ60CL/209624 |
| 专题 | 理学院_物理系 |
| 作者单位 | 1.Department of Physics and Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressure,Southern University of Science and Technology,Shenzhen,518055,China 2.College of Science,Institute of Functional Materials,State Key Laboratory for Modification of Chemical Fibers and Polymer Materials,Donghua University,201620,China 3.Key Laboratory for Neutron Physics,Institute of Nuclear Physics and Chemistry,China Academy of Engineering Physics,China 4.Department of Physics and Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressure, Southern University of Science and Technology, Shenzhen 518055, China. wangsm@sustech.edu.cn and Key Laboratory of Extreme Conditions Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China 5.Key Laboratory of Extreme Conditions Physics,Institute of Physics,Chinese Academy of Sciences,100190,China 6.College of Science,Institute of Functional Materials,State Key Laboratory for Modification of Chemical Fibers and Polymer Materials,Donghua University,201620,China 7.Department of Physics and Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressure,Southern University of Science and Technology,Shenzhen,518055,China |
| 第一作者单位 | 物理系 |
| 通讯作者单位 | 物理系 |
| 第一作者的第一单位 | 物理系 |
| 推荐引用方式 GB/T 7714 |
Ahmad，Azkar Saeed,Liang,Yongcheng,Dong，Mingdong,et al. Pressure-driven switching of magnetism in layered CrCl3[J]. Nanoscale,2020,12(45):22935-22944.
|
| APA |
Ahmad，Azkar Saeed.,Liang,Yongcheng.,Dong，Mingdong.,Zhou，Xuefeng.,Fang，Leiming.,...&Wang，Shanmin.(2020).Pressure-driven switching of magnetism in layered CrCl3.Nanoscale,12(45),22935-22944.
|
| MLA |
Ahmad，Azkar Saeed,et al."Pressure-driven switching of magnetism in layered CrCl3".Nanoscale 12.45(2020):22935-22944.
|
| 条目包含的文件 | 条目无相关文件。 | |||||
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