| 题名 | A medium-range structure motif linking amorphous and crystalline states |
| 作者 | Lan，Si1,2  ; Zhu，Li3; Wu，Zhenduo4; Gu，Lin5; Zhang，Qinghua5; Kong，Huihui1; Liu，Jizi1; Song，Ruoyu6; Liu，Sinan1; Sha，Gang1; Wang，Yingang3; Liu，Qi2; Liu，Wei1; Wang，Peiyi7 ; Liu，Chain Tsuan8; Ren，Yang9; Wang，Xun Li2,10; Lan，Si11,12; Zhu，Li13; Wu，Zhenduo14; Gu，Lin15; Zhang，Qinghua15; Kong，Huihui11; Liu，Jizi11; Song，Ruoyu16; Liu，Sinan11; Sha，Gang11; Wang，Yingang13; Liu，Qi12; Liu，Wei11; Wang，Peiyi17; Liu，Chain Tsuan18; Ren，Yang19; Wang，Xun Li12,20; Lan，Si21,22; Zhu，Li23; Wu，Zhenduo24; Gu，Lin25; Zhang，Qinghua25; Kong，Huihui21; Liu，Jizi21; Song，Ruoyu26; Liu，Sinan21; Sha，Gang21; Wang，Yingang23; Liu，Qi22; Liu，Wei21; Wang，Peiyi27; Liu，Chain Tsuan28; Ren，Yang29; Wang，Xun Li22,30; Lan，Si31,32; Zhu，Li33; Wu，Zhenduo34; Gu，Lin35; Zhang，Qinghua35; Kong，Huihui31; Liu，Jizi31; Song，Ruoyu36; Liu，Sinan31; Sha，Gang31; Wang，Yingang33; Liu，Qi32; Liu，Wei31; Wang，Peiyi37; Liu，Chain Tsuan38; Ren，Yang39; Wang，Xun Li32,40
|
| 通讯作者 | Lan，Si; Lan，Si; Lan，Si; Lan，Si |
| 发表日期 | 2021
|
| DOI | |
| 发表期刊 | |
| ISSN | 1476-1122
|
| EISSN | 1476-4660
|
| 卷号 | 20页码:1347-1352 |
| 摘要 | Amorphous materials have no long-range order, but there are ordered structures at short range (2–5 Å), medium range (5–20 Å) and even longer length scales. While regular and semiregular polyhedra are often found as short-range ordering in amorphous materials, the nature of medium-range order has remained elusive. Consequently, it is difficult to determine whether there exists any structural link at medium range or longer length scales between the amorphous material and its crystalline counterparts. Moreover, an amorphous material often crystallizes into a phase of different composition, with very different underlying structural building blocks, further compounding the issue. Here, we capture an intermediate crystalline cubic phase in a Pd-Ni-P amorphous alloy and reveal the structure of the medium-range order, a six-membered tricapped trigonal prism cluster (6M-TTP) with a length scale of 12.5 Å. We find that the 6M-TTP can pack periodically to several tens of nanometres to form the cube phase. Our experimental observations provide evidence of a structural link between the amorphous and crystalline phases in a Pd-Ni-P alloy at the medium-range length scale and suggest that it is the connectivity of the 6M-TTP clusters that distinguishes the crystalline and amorphous phases. These findings will shed light on the structure of amorphous materials at extended length scales beyond that of short-range order. |
| 相关链接 | [Scopus记录] |
| 收录类别 | |
| 语种 | 英语
|
| 重要成果 | NI论文
|
| 学校署名 | 其他
|
| WOS记录号 | WOS:000652442900003
|
| EI入藏号 | 20212110408183
|
| EI主题词 | Nickel alloys
; Palladium alloys
|
| EI分类号 | Metallurgy and Metallography:531
; Precious Metals:547.1
; Nickel Alloys:548.2
|
| ESI学科分类 | MATERIALS SCIENCE
|
| Scopus记录号 | 2-s2.0-85106241722
|
| 来源库 | Scopus
|
| 引用统计 |
被引频次[WOS]：124
|
| 成果类型 | 期刊论文 |
| 条目标识符 | http://sustech.caswiz.com/handle/2SGJ60CL/229651 |
| 专题 | 冷冻电镜中心 |
| 作者单位 | 1.Herbert Gleiter Institute of Nanoscience,School of Materials Science and Engineering,Nanjing University of Science and Technology,Nanjing,China 2.Department of Physics,City University of Hong Kong,Kowloon,Hong Kong 3.College of Materials Science and Technology,Nanjing University of Aeronautics and Astronautics,Nanjing,China 4.Center for Neutron Scattering and Applied Physics,City University of Hong Kong Dongguan Research Institute,Dongguan,China 5.Beijing National Laboratory for Condensed Matter Physics and Collaborative Innovation Center of Quantum Matter,Institute of Physics,Chinese Academy of Sciences,Beijing,China 6.Woodruff School of Mechanical Engineering,Georgia Institute of Technology,Atlanta,United States 7.SUSTech Cryo-EM Facility Center,Southern University of Science and Technology,Shenzhen,China 8.Center for Advanced Structural Materials & Department of Materials Science and Engineering,City University of Hong Kong,Kowloon,Hong Kong 9.X-ray Science Division,Argonne National Laboratory,Argonne,United States 10.Center for Neutron Scattering,City University of Hong Kong Shenzhen Research Institute,Shenzhen,China 11.Herbert Gleiter Institute of Nanoscience,School of Materials Science and Engineering,Nanjing University of Science and Technology,Nanjing,China 12.Department of Physics,City University of Hong Kong,Kowloon,Hong Kong 13.College of Materials Science and Technology,Nanjing University of Aeronautics and Astronautics,Nanjing,China 14.Center for Neutron Scattering and Applied Physics,City University of Hong Kong Dongguan Research Institute,Dongguan,China 15.Beijing National Laboratory for Condensed Matter Physics and Collaborative Innovation Center of Quantum Matter,Institute of Physics,Chinese Academy of Sciences,Beijing,China 16.Woodruff School of Mechanical Engineering,Georgia Institute of Technology,Atlanta,United States 17.SUSTech Cryo-EM Facility Center,Southern University of Science and Technology,Shenzhen,China 18.Center for Advanced Structural Materials & Department of Materials Science and Engineering,City University of Hong Kong,Kowloon,Hong Kong 19.X-ray Science Division,Argonne National Laboratory,Argonne,United States 20.Center for Neutron Scattering,City University of Hong Kong Shenzhen Research Institute,Shenzhen,China 21.Herbert Gleiter Institute of Nanoscience,School of Materials Science and Engineering,Nanjing University of Science and Technology,Nanjing,China 22.Department of Physics,City University of Hong Kong,Kowloon,Hong Kong 23.College of Materials Science and Technology,Nanjing University of Aeronautics and Astronautics,Nanjing,China 24.Center for Neutron Scattering and Applied Physics,City University of Hong Kong Dongguan Research Institute,Dongguan,China 25.Beijing National Laboratory for Condensed Matter Physics and Collaborative Innovation Center of Quantum Matter,Institute of Physics,Chinese Academy of Sciences,Beijing,China 26.Woodruff School of Mechanical Engineering,Georgia Institute of Technology,Atlanta,United States 27.SUSTech Cryo-EM Facility Center,Southern University of Science and Technology,Shenzhen,China 28.Center for Advanced Structural Materials & Department of Materials Science and Engineering,City University of Hong Kong,Kowloon,Hong Kong 29.X-ray Science Division,Argonne National Laboratory,Argonne,United States 30.Center for Neutron Scattering,City University of Hong Kong Shenzhen Research Institute,Shenzhen,China 31.Herbert Gleiter Institute of Nanoscience,School of Materials Science and Engineering,Nanjing University of Science and Technology,Nanjing,China 32.Department of Physics,City University of Hong Kong,Kowloon,Hong Kong 33.College of Materials Science and Technology,Nanjing University of Aeronautics and Astronautics,Nanjing,China 34.Center for Neutron Scattering and Applied Physics,City University of Hong Kong Dongguan Research Institute,Dongguan,China 35.Beijing National Laboratory for Condensed Matter Physics and Collaborative Innovation Center of Quantum Matter,Institute of Physics,Chinese Academy of Sciences,Beijing,China 36.Woodruff School of Mechanical Engineering,Georgia Institute of Technology,Atlanta,United States 37.SUSTech Cryo-EM Facility Center,Southern University of Science and Technology,Shenzhen,China 38.Center for Advanced Structural Materials & Department of Materials Science and Engineering,City University of Hong Kong,Kowloon,Hong Kong 39.X-ray Science Division,Argonne National Laboratory,Argonne,United States 40.Center for Neutron Scattering,City University of Hong Kong Shenzhen Research Institute,Shenzhen,China |
| 推荐引用方式 GB/T 7714 |
Lan，Si,Zhu，Li,Wu，Zhenduo,et al. A medium-range structure motif linking amorphous and crystalline states[J]. NATURE MATERIALS,2021,20:1347-1352.
|
| APA |
Lan，Si.,Zhu，Li.,Wu，Zhenduo.,Gu，Lin.,Zhang，Qinghua.,...&Wang，Xun Li.(2021).A medium-range structure motif linking amorphous and crystalline states.NATURE MATERIALS,20,1347-1352.
|
| MLA |
Lan，Si,et al."A medium-range structure motif linking amorphous and crystalline states".NATURE MATERIALS 20(2021):1347-1352.
|
| 条目包含的文件 | ||||||
| 文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | 操作 | |
| A medium-range struc（16564KB） | -- | -- | 限制开放 | -- | ||
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。
修改评论