In-depth Understanding of the Effects of Intramolecular Charge Transfer on Carbon Nitride Based Photocatalysts†

Sun，Zongzhao1; Tan，Yueyang1,2; Wan，Jianyong1; Huang，Limin1,3,4,5

2021-07-01

10.1002/cjoc.202000743

CHINESE JOURNAL OF CHEMISTRY   影响因子和分区

1001-604X

1614-7065

Intramolecular charge transfer (ICT) derived from a donor-acceptor system has been applied for years to enhance the charge mobility in the field of organic photovoltaics and chemical sensing. Similar strategies have gradually been developed in polymeric graphitic carbon nitride (GCN) photocatalytic systems for promoting the light absorption and charge separation. However, there are no reviews focusing on the effects of ICT after the modification of GCN so far. Herein, we summarize some typical literature on GCN engineering to expound profoundly the roles of ICT in electronic properties regulation in terms of in-situ formation and molecular coupling. At last, some important perspectives are also proposed. This review will deepen understanding of the traditional theory for a new recognition among such many methods to improve the performance of GCN.

Donor-acceptor systems Energy conversion Graphitic carbon nitride Intramolecular charge transfer Photocatalysis

SCI

英语

第一 ; 通讯

WOS:000663032500038

CHEMISTRY

2-s2.0-85108011937

Scopus

1.Department of Chemistry,Southern University of Science and Technology,Shenzhen,518055,China
2.Harbin Institute of Technology,Harbin,150001,China
3.Guangdong Provincial Key Laboratory of Energy Materials for Electric Power,Southern University of Science and Technology,Shenzhen,518055,China
4.Guangdong-Hong Kong-Macao Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices,Southern University of Science and Technology,Shenzhen,518055,China
5.Shenzhen Key Laboratory of Solid State Batteries,Southern University of Science and Technology,Shenzhen,518055,China

Sun，Zongzhao,Tan，Yueyang,Wan，Jianyong,等. In-depth Understanding of the Effects of Intramolecular Charge Transfer on Carbon Nitride Based Photocatalysts†[J]. CHINESE JOURNAL OF CHEMISTRY,2021,39(7):2044-2053.

Sun，Zongzhao,Tan，Yueyang,Wan，Jianyong,&Huang，Limin.(2021).In-depth Understanding of the Effects of Intramolecular Charge Transfer on Carbon Nitride Based Photocatalysts†.CHINESE JOURNAL OF CHEMISTRY,39(7),2044-2053.

Sun，Zongzhao,et al."In-depth Understanding of the Effects of Intramolecular Charge Transfer on Carbon Nitride Based Photocatalysts†".CHINESE JOURNAL OF CHEMISTRY 39.7(2021):2044-2053.