| 题名 | Spatial and temporal scales of variability for indoor air constituents |
| 作者 | Lakey，Pascale S.J.1; Won，Youngbo2; Shaw，David3; Østerstrøm，Freja F.3; Mattila，James4; Reidy，Emily5; Bottorff，Brandon5; Rosales，Colleen5; Wang，Chen6,13  ; Ampollini，Laura7; Zhou，Shan8,9; Novoselac，Atila10; Kahan，Tara F.8,11; DeCarlo，Peter F.12; Abbatt，Jonathan P.D.6; Stevens，Philip S.5; Farmer，Delphine K.4; Carslaw，Nicola3; Rim，Donghyun2; Shiraiwa，Manabu1
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| 通讯作者 | Shiraiwa，Manabu |
| 发表日期 | 2021-12-01
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| DOI | |
| 发表期刊 | |
| ISSN | 2399-3669
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| EISSN | 2399-3669
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| 卷号 | 4期号:1 |
| 摘要 | Historically air constituents have been assumed to be well mixed in indoor environments, with single point measurements and box modeling representing a room or a house. Here we demonstrate that this fundamental assumption needs to be revisited through advanced model simulations and extensive measurements of bleach cleaning. We show that inorganic chlorinated products, such as hypochlorous acid and chloramines generated via multiphase reactions, exhibit spatial and vertical concentration gradients in a room, with short-lived ⋅OH radicals confined to sunlit zones, close to windows. Spatial and temporal scales of indoor constituents are modulated by rates of chemical reactions, surface interactions and building ventilation, providing critical insights for better assessments of human exposure to hazardous pollutants, as well as the transport of indoor chemicals outdoors. |
| 相关链接 | [Scopus记录] |
| 收录类别 | |
| 语种 | 英语
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| 学校署名 | 其他
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| 资助项目 | Alfred P. Sloan Foundation[
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| WOS研究方向 | Chemistry
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| WOS类目 | Chemistry, Multidisciplinary
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| WOS记录号 | WOS:000685304400001
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| 出版者 | |
| Scopus记录号 | 2-s2.0-85112729458
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| 来源库 | Scopus
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| 引用统计 |
被引频次[WOS]：25
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| 成果类型 | 期刊论文 |
| 条目标识符 | http://sustech.caswiz.com/handle/2SGJ60CL/242979 |
| 专题 | 工学院_环境科学与工程学院 |
| 作者单位 | 1.Department of Chemistry,University of California,Irvine,Irvine,United States 2.Department of Architectural Engineering,Pennsylvania State University,University Park,United States 3.Department of Environment and Geography,University of York,York,United Kingdom 4.Department of Chemistry,Colorado State University,Fort Collins,United States 5.Department of Chemistry and O’Neill School of Public and Environmental Affairs,Indiana University Bloomington,Bloomington,United States 6.Department of Chemistry,University of Toronto,Toronto,Canada 7.Department of Civil,Architectural,and Environmental Engineering,Drexel University,Philadelphia,United States 8.Department of Chemistry,Syracuse University,Syracuse,United States 9.Department of Civil and Environmental Engineering,Rice University,Houston,United States 10.Department of Civil,Architectural,and Environmental Engineering,University of Texas,Austin,United States 11.Department of Chemistry,University of Saskatchewan,Saskatoon,Canada 12.Department of Environmental Health and Engineering,Johns Hopkins University,Baltimore,United States 13.School of Environmental Science and Engineering,Southern University of Science and Technology,Shenzhen,518055,China |
| 推荐引用方式 GB/T 7714 |
Lakey，Pascale S.J.,Won，Youngbo,Shaw，David,et al. Spatial and temporal scales of variability for indoor air constituents[J]. Communications Chemistry,2021,4(1).
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| APA |
Lakey，Pascale S.J..,Won，Youngbo.,Shaw，David.,Østerstrøm，Freja F..,Mattila，James.,...&Shiraiwa，Manabu.(2021).Spatial and temporal scales of variability for indoor air constituents.Communications Chemistry,4(1).
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| MLA |
Lakey，Pascale S.J.,et al."Spatial and temporal scales of variability for indoor air constituents".Communications Chemistry 4.1(2021).
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| 条目包含的文件 | ||||||
| 文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | 操作 | |
| Spatial and Temporal（1784KB） | -- | -- | 开放获取 | -- | 浏览 | |
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