中文版 | English
题名

A wafer-scale two-dimensional platinum monosulfide ultrathin film via metal sulfurization for high performance photoelectronics

作者
通讯作者Pang, Jinbo; Yang, Feng; Wang, Xiao
共同第一作者Pang, Jinbo; Wang, Yanhao; Yang, Xiaoxin; Zhang, Lei
发表日期
2022
DOI
发表期刊
EISSN
2633-5409
卷号3页码:1497–1505
摘要

2D nonlayered materials have attracted enormous research interests due to their novel physical and chemical properties with confined dimensions. Platinum monosulfide as one of the most common platinum-group minerals has been less studied due to either the low purity in the natural product or the extremely high-pressure conditions for synthesis. Recently, platinum monosulfide (PtS) 2D membranes have emerged as rising-star materials for fundamental Raman and X-ray photoelectron spectral analysis as well as device exploration. However, a large-area homogeneous synthesis route has not yet been proposed and released. In this communication, we report a facile metal sulfurization strategy for the synthesis of a 4-inch wafer-scale PtS film. Enhanced characterization tools have been employed for thorough analysis of the crystal structure, chemical environment, vibrational modes, and atomic configuration. Furthermore, through theoretical calculations the phase diagram of the Pt-S compound has been plotted for showing the successful formation of PtS in our synthesis conditions. Eventually, a high-quality PtS film has been reflected in device demonstration by a photodetector. Our approach may shed light on the mass production of PtS films with precise control of their thickness and homogeneity as well as van der Waals heterostructures and related electronic devices.

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语种
英语
学校署名
通讯
资助项目
National Natural Science Foundation of China (NSFC)[51802116] ; Natural Science Foundation of Shandong Province[ZR2019BEM040] ; State Key Laboratory of Biobased Material and Green Papermaking (Qilu University of Technology, Shandong Academy of Sciences)[GZKF202107] ; National Key Research and Development Program of China from the Ministry of Science and Technology (MOST) of China[2021YFA0717400] ; Natural Science Foundation for Distinguished Young Scientists of Shandong Province[JQ201814] ; Project of
WOS研究方向
Materials Science
WOS类目
Materials Science, Multidisciplinary
WOS记录号
WOS:000742408200001
出版者
来源库
Web of Science
出版状态
正式出版
引用统计
被引频次[WOS]:16
成果类型期刊论文
条目标识符http://sustech.caswiz.com/handle/2SGJ60CL/272494
专题理学院_化学系
作者单位
1.Univ Jinan, Collaborat Innovat Ctr Technol & Equipment Biol D, Inst Adv Interdisciplinary Res iAIR, Jinan 250022, Shandong, Peoples R China
2.Shandong Univ, Inst Marine Sci & Technol, Qingdao 266237, Shandong, Peoples R China
3.Chinese Acad Sci, Interdisciplinary Res Ctr, Shanghai Adv Res Inst, 99 Haike Rd,Zhangjiang Hitech Pk, Shanghai 201210, Peoples R China
4.Univ Chinese Acad Sci, Sch Microelect, 19 Yuquan Rd, Beijing 100049, Peoples R China
5.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen Key Lab Nanobiomech, Shenzhen 518055, Peoples R China
6.Department of Chemistry, Southern University of Science and Technology, Shenzhen, 518055, China
7.Tech Univ Dresden, Inst Mat Sci, D-01069 Dresden, Germany
8.Tech Univ Dresden, Max Bergmann Ctr Biomat, D-01069 Dresden, Germany
9.Tech Univ Dresden, Ctr Adv Elect Dresden, D-01069 Dresden, Germany
10.Shandong Univ, Ctr Bio & Micro Nano Funct Mat, State Key Lab Crystal Mat, 27 Shandanan Rd, Jinan 250100, Peoples R China
11.Soochow Univ, Key Lab Adv Carbon Mat & Wearable Energy Technol, Coll Energy, Soochow Inst Energy & Mat Innovat, Chinasuzhou 215006, Peoples R China
12.Polish Acad Sci, Ctr Polymer & Carbon Mat, M Curie Sklodowskiej 34, PL-41819 Zabrze, Poland
13.IFW Dresden, Inst Complex Mat, 20 Helmholtz Str, D-01069 Dresden, Germany
14.VSB Tech Univ Ostrava, Inst Environm Technol, 17 Listopadu 15, Ostrava 70833, Czech Republic
15.Tech Univt Dresden, Dresden Ctr Computat Mat Sci, D-01062 Dresden, Germany
16.Tech Univ Dresden, Dresden Ctr Intelligent Mat DCIM, D-01062 Dresden, Germany
通讯作者单位化学系
推荐引用方式
GB/T 7714
Pang, Jinbo,Wang, Yanhao,Yang, Xiaoxin,et al. A wafer-scale two-dimensional platinum monosulfide ultrathin film via metal sulfurization for high performance photoelectronics[J]. MATERIALS ADVANCES,2022,3:1497–1505.
APA
Pang, Jinbo.,Wang, Yanhao.,Yang, Xiaoxin.,Zhang, Lei.,Li, Yufen.,...&Ruemmeli, Mark H..(2022).A wafer-scale two-dimensional platinum monosulfide ultrathin film via metal sulfurization for high performance photoelectronics.MATERIALS ADVANCES,3,1497–1505.
MLA
Pang, Jinbo,et al."A wafer-scale two-dimensional platinum monosulfide ultrathin film via metal sulfurization for high performance photoelectronics".MATERIALS ADVANCES 3(2022):1497–1505.
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