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题名

Vapor-Phase Deposition of Highly Luminescent Embedded Perovskite Nanocrystals

作者
通讯作者Luo,Deying
发表日期
2022
DOI
发表期刊
ISSN
2195-1071
EISSN
2195-1071
卷号10
摘要
Vapor-phase deposition (VPD), a process that can be readily scaled up for mass production, provides a cost-effective approach to manufacture perovskite light-emitting diodes (LEDs). The progress in device efficiency, however, has been stagnant, owing largely to the poor photoluminescence quantum yields (PLQYs) of the VPD materials. Herein, a holistic fabrication strategy is reported that can stabilize the otherwise thermodynamically unstable cubic-phase through the deposition of a CsBr-rich termination on top of the CsPbBr films. The enhanced film reduces the electronic defects considerably resulting in near-unity PLQY of the VPD-based perovskites. To understand the mechanism of the improved VPD-CsPbBr perovskite, advanced optical probing techniques and structural characterizations are used. For device application, the LEDs made from the VPD perovskites yield a bright luminance of ≈15 000 cd m at 523 nm with a sharp full width at half maximum (FWHM) of 18 nm.
关键词
相关链接[Scopus记录]
收录类别
SCI ; EI
语种
英语
学校署名
其他
资助项目
Research and Application of Key Technologies of GaN-based Power Devices on Si Substrate[2019B010128001] ; Research on key technologies for optimization of IoT chips and product development[2019B010142001] ; Study and optimization of electrostatic discharge mechanism for GaN HEMT devices[JCYJ20180305180619573] ; Research of AlGaN HEMT MEMS sensor for work in extreme environment[JCYJ20170412153356899]
WOS研究方向
Materials Science ; Optics
WOS类目
Materials Science, Multidisciplinary ; Optics
WOS记录号
WOS:000778948600001
出版者
EI入藏号
20221511937317
EI主题词
Bromine compounds ; Cesium compounds ; Cost effectiveness ; Lead compounds ; Light emitting diodes ; Nanocrystals ; Vapor deposition
EI分类号
Minerals:482.2 ; Semiconductor Devices and Integrated Circuits:714.2 ; Nanotechnology:761 ; Industrial Economics:911.2 ; Crystalline Solids:933.1
Scopus记录号
2-s2.0-85127601182
来源库
Scopus
引用统计
被引频次[WOS]:1
成果类型期刊论文
条目标识符http://sustech.caswiz.com/handle/2SGJ60CL/329634
专题工学院_深港微电子学院
工学院_材料科学与工程系
作者单位
1.Department of Physics,Center for Optoelectronics Engineering Research,Yunnan University,Kunming,650091,China
2.Department of Materials Science and Engineering,University of Toronto,Toronto,M5G 3E4,Canada
3.Department of Chemistry,University of Toronto,Toronto,M5S 3H6,Canada
4.Department of Electrical and Computer Engineering,University of Toronto,Toronto,M5S 3G8,Canada
5.School of Microelectronics,Southern University of Science and Technology,Shenzhen,518055,China
推荐引用方式
GB/T 7714
Li,Xiaoyue,Luo,Deying,Green,Philippe B.,et al. Vapor-Phase Deposition of Highly Luminescent Embedded Perovskite Nanocrystals[J]. Advanced Optical Materials,2022,10.
APA
Li,Xiaoyue.,Luo,Deying.,Green,Philippe B..,Qiu,Chenyue.,Wei,Mingyang.,...&Lu,Zheng Hong.(2022).Vapor-Phase Deposition of Highly Luminescent Embedded Perovskite Nanocrystals.Advanced Optical Materials,10.
MLA
Li,Xiaoyue,et al."Vapor-Phase Deposition of Highly Luminescent Embedded Perovskite Nanocrystals".Advanced Optical Materials 10(2022).
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