Directional emissions from perovskite nanocrystals thin film enabled by metasurface integration through one step spin-coating process

Li, Kexue1; Zhang, Xuanyu2; Ni, Peinan3; Liu, Juncheng1; Lin, Fengyuan1; Man, Xu1; Cai, Wenfeng2; Liu, Jianxun2; Liu, Yanjun2; Chen, Rui2; Wei, Zhipeng1

2023-03-01

10.1007/s12274-023-5439-y

Nano Research   影响因子和分区

1998-0124

1998-0000

Advances in thin film light-emitting devices have fueled the rapid growth of a new class of solid-state lighting devices, featuring low fabrication cost, high quantum efficiency, and broadband spectrum coverage, etc. In contrast to the conventional inorganic semiconductors that rely on lattice matched high crystalline quality substrate, solution processable thin films eliminate the dependence on the substrate, which is highly desired for the ease and versatility of integrations with foreign medium. By taking this advantage, this work developed an ultracompact solution to control the directionality of thin film emitters using integrated dielectric metasurface through one step spin-coating process. As a proof of concept, directional emissions from perovskite nanocrystal thin film, including collimated light emissions and two-dimensional beam steering, are experimentally demonstrated. Notably, our approach, where light emitters were integrated on the back side of substrate after the fabrication of metasurface, judiciously avoids any potential degradation of material optical quality caused by the multi-step nanofabrication. Therefore, it can serve as a generalized scheme to engage the advantageous properties of dielectric metasurface, including the compactness, high efficiency, and beam controllability with the emerging thin film light-emitting diodes (LEDs), which is applicable to a wide range of solution processable materials, including organic light-emitting diodes, quantum-dot light emitting diodes, polymer LEDs, and perovskite LEDs, opening up new pathways to develop low-cost and ultra-compact solid state light sources with versatile beams characteristics.

solid state light source perovskite light-emitting diodes (LEDs) metasurface integrations on-chip beam shaping beam steering

SCI ; EI

英语

其他

National Natural Science Foundation of China["11804335","61904017","12074045","62174079"] ; Science, Technology and Innovation Commission of Shenzhen Municipality["JCYJ20210324120204011","KQTD2015071710313656"] ; H2020 Research and Innovation Program (Marie Sklodowska-Curie Individual Fellowship)[101027383]

Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics

Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied

WOS:000947308100001

TSINGHUA UNIV PRESS

20231113698753

Coatings ; Costs ; Dielectric materials ; Efficiency ; Nanocrystals ; Organic light emitting diodes (OLED) ; Perovskite solar cells ; Semiconductor quantum dots ; Substrates ; Thin films

Minerals:482.2 ; Solar Cells:702.3 ; Dielectric Materials:708.1 ; Semiconductor Devices and Integrated Circuits:714.2 ; Nanotechnology:761 ; Coating Materials:813.2 ; Cost and Value Engineering; Industrial Economics:911 ; Production Engineering:913.1 ; Crystalline Solids:933.1

Web of Science

1.Changchun Univ Sci & Technol, Sch Phys, State Key Lab High Power Semicond Laser, Changchun 130022, Peoples R China
2.Southern Univ Sci & Technol, Dept Elect & Elect Engn, Shenzhen 518055, Peoples R China
3.Chalmers Univ Technol, Dept Microtechnol & Nanosci, Photon Lab, SE-41296 Gothenburg, Sweden

Li, Kexue,Zhang, Xuanyu,Ni, Peinan,et al. Directional emissions from perovskite nanocrystals thin film enabled by metasurface integration through one step spin-coating process[J]. Nano Research,2023,16(5):7646-7653.

Li, Kexue.,Zhang, Xuanyu.,Ni, Peinan.,Liu, Juncheng.,Lin, Fengyuan.,...&Wei, Zhipeng.(2023).Directional emissions from perovskite nanocrystals thin film enabled by metasurface integration through one step spin-coating process.Nano Research,16(5),7646-7653.

Li, Kexue,et al."Directional emissions from perovskite nanocrystals thin film enabled by metasurface integration through one step spin-coating process".Nano Research 16.5(2023):7646-7653.