Microindentation analysis of mechanical properties evolution during an artificial hydrocarbon generation process

Zhang, Pengyu1,2; Zhao, Junliang3; Zhang, Dongxiao3; Xia, Zunyi1,2

2023-07-01

10.1016/j.jgsce.2023.205003

GAS SCIENCE AND ENGINEERING   影响因子和分区

2949-9097

2949-9089

The last decade witnessed rapid growth of shale oil and gas production. Increasing numbers of shale reservoirs have been explored and developed. Since hydrocarbon generation is an important process in forming a shale reservoir, it has attracted great attention from researchers. However, previous works mainly focus on geochemical changes during the hydrocarbon generation process, and investigations of the change of other parameters are insufficient. In this study, we intend to fill this gap in the literature by examining the mechanical properties evolution of organic-rich shales during an artificial hydrocarbon generation experiment. Continuous stiffness measurement (CSM) and microindentation test are used to measure the mechanical properties of rocks. The result of CSM shows the influence of indentation depth on Young's modulus. Three stages are identified, and a displacement of 4000 nm-6000 nm is determined to be appropriate for measuring bulk mechanical properties. Microindentation results of shales at different hydrocarbon generation stages exhibit a hill-like trend. The Young's modulus with an initial value of 42.15 GPa increases as the hydrocarbon generation proceeds, reaches a maximum value of 46.49 GPa, and then begins to decrease and reaches the lowest value of 37.41 GPa. Indentation hardness and estimated fracture toughness by an energy-based method show similar trends to Young's modulus. Scanning electron microscope observation of post-hydrocarbon-generation samples may provide an explanation of the hill-like trend.

Organic-rich shale Hydrocarbon generation Continuous stiffness measurement Microindentation Mechanical properties

SCI ; EI

英语

通讯

Shenzhen Key Laboratory of Natural Gas Hydrates[ZDSYS20200421111201738]

Energy & Fuels ; Engineering

Energy & Fuels ; Engineering, Chemical

WOS:001049398000001

ELSEVIER

20233714727827

Ductile fracture ; Fracture toughness ; Hydrocarbons ; Indentation ; Scanning electron microscopy ; Stiffness

Organic Compounds:804.1 ; Materials Science:951

Web of Science

1.Peking Univ, Coll Engn, BIC ESAT, ERE, Beijing, Peoples R China
2.Peking Univ, Coll Engn, SKLTCS, Beijing, Peoples R China
3.Southern Univ Sci & Technol, Shenzhen Key Lab Nat Gas Hydrates, Shenzhen 518055, Peoples R China

Zhang, Pengyu,Zhao, Junliang,Zhang, Dongxiao,et al. Microindentation analysis of mechanical properties evolution during an artificial hydrocarbon generation process[J]. GAS SCIENCE AND ENGINEERING,2023,115.

Zhang, Pengyu,Zhao, Junliang,Zhang, Dongxiao,&Xia, Zunyi.(2023).Microindentation analysis of mechanical properties evolution during an artificial hydrocarbon generation process.GAS SCIENCE AND ENGINEERING,115.

Zhang, Pengyu,et al."Microindentation analysis of mechanical properties evolution during an artificial hydrocarbon generation process".GAS SCIENCE AND ENGINEERING 115(2023).