南方科技大学知识苑(SUSTech KC): Advances and challenges in single-site catalysts towards electrochemical CO<sub>2</sub> methanation

题名	Advances and challenges in single-site catalysts towards electrochemical CO₂ methanation
作者	Zhu, Jiexin 1,2; Lv, Lei 1; Zaman, Shahid5 ; Chen, Xingbao 1; Dai, Yuhang 1,2; Chen, Shenghua 3; He, Guanjie 2; Wang, Dingsheng 4; Mai, Liqiang 1
通讯作者	Chen, Shenghua; Wang, Dingsheng; Mai, Liqiang
发表日期	2023-09-01
DOI	10.1039/d3ee02196
发表期刊	ENERGY & ENVIRONMENTAL SCIENCE 影响因子和分区
ISSN	1754-5692
EISSN	1754-5706
摘要	Electrochemical CO2 reduction to a valuable product is a sustainable and economical method towards carbon neutralization. Among the different products of the electrochemical CO2 reduction reaction (CO2RR), methane is an excellent energy carrier with a high combustion heat. However, for higher methane product selectivity it is crucial to avoid C-C coupling that leads to multi-carbon products. Thus, single-site catalysts (SSCs) with a single active site are ideal candidates. This review summarizes and discusses the current research progress and future application prospects of electrochemical CO2 methanation on SSCs. The CO2 methanation mechanism and primary activity descriptors are discussed in detail with an extensive overview of the coordination structure and design of SSCs, as well as their several in situ characterization methods for tracking the structural changes in SSCs. This review provides insights into the further exploitation of SSCs for selective CO2 methanation that inspires the rational design of SSCs in electrochemical CO2 methanation research.
相关链接	[来源记录]
收录类别	SCI
语种	英语
学校署名	其他
资助项目	L. M. acknowledges the National Key Research and Development Program of China (2020YFA0715000), the National Natural Science Foundation of China (51832004, 52127816), and the National Energy-Saving and Low-Carbon Materials Production and Application Demons[2020YFA0715000] ; National Key Research and Development Program of China["51832004","52127816"] ; National Natural Science Foundation of China[TC220H06N] ; National Energy-Saving and Low-Carbon Materials Production and Application Demonstration Platform Program[71211223010707]
WOS研究方向	Chemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS类目	Chemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS记录号	WOS:001075167900001
出版者	ROYAL SOC CHEMISTRY
来源库	Web of Science
引用统计	被引频次[WOS]：22
成果类型	期刊论文
条目标识符	http://sustech.caswiz.com/handle/2SGJ60CL/575810
专题	工学院_机械与能源工程系
作者单位	1.Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China 2.UCL, Dept Chem Engn, Electrochem Innovat Lab, London WC1E 7JE, England 3.Xi An Jiao Tong Univ, Sch Chem Engn & Technol, Natl Innovat Platform Ctr Ind Educ Integrat Energy, Xian 710049, Peoples R China 4.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China 5.Southern Univ Sci & Technol, Dept Mech & Energy Engn, Shenzhen 518055, Peoples R China
推荐引用方式 GB/T 7714	Zhu, Jiexin,Lv, Lei,Zaman, Shahid,et al. Advances and challenges in single-site catalysts towards electrochemical CO₂ methanation[J]. ENERGY & ENVIRONMENTAL SCIENCE,2023.
APA	Zhu, Jiexin.,Lv, Lei.,Zaman, Shahid.,Chen, Xingbao.,Dai, Yuhang.,...&Mai, Liqiang.(2023).Advances and challenges in single-site catalysts towards electrochemical CO₂ methanation.ENERGY & ENVIRONMENTAL SCIENCE.
MLA	Zhu, Jiexin,et al."Advances and challenges in single-site catalysts towards electrochemical CO₂ methanation".ENERGY & ENVIRONMENTAL SCIENCE (2023).