南方科技大学知识苑(SUSTech KC): Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles

题名	Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles
作者	Liu, Yu-Feng 1; Hu, Qi-Long 1; Chen, Xue-Jiao 1; Li, Ke 1; Luo, Pei2 ; Yang, Guo-Ping 1
通讯作者	Li, Ke; Luo, Pei; Yang, Guo-Ping
发表日期	2023-12-01
DOI	10.1007/s12598-023-02532-5
发表期刊	RARE METALS 影响因子和分区
ISSN	1001-0521
EISSN	1867-7185
摘要	Diversified synthetic strategies are extremely important for the structural diversity of uranium-containing polyoxometalates (U-POMs) and their functional expansion. Herein, two sandwich-type U-POMs were reported, which are Na5.6K6.4[(UO2)(H2O)(TeW9O33)](2)21H(2)O (UTeW9) and Na8.9K2.7H1.19[K-0.79(UO2)(2.21)(PW9O34)(2)]12H(2)O (UPW9) using in-situ strategy and lacunary precursor strategy, respectively. UTeW9 shows a typical Keggin-type open or half-sandwich configuration. UPW9 shows a typical Keggin-type sandwiched structure containing significant disorders of K(I) and uranyl ions with a triangular configuration. In addition, UTeW9 exhibits high efficiency in the catalyzed condensation of various o-arylenediamines and aldehydes for the aerobic synthesis of benzimidazoles with excellent yield.
相关链接	[来源记录]
收录类别	SCI ; EI
语种	英语
学校署名	通讯
资助项目	National Natural Science Foundation of China[22001034] ; National Natural Science Foundation of China[20212BAB213001]
WOS研究方向	Materials Science ; Metallurgy & Metallurgical Engineering
WOS类目	Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS记录号	WOS:001131843200001
出版者	NONFERROUS METALS SOC CHINA
ESI学科分类	MATERIALS SCIENCE
来源库	Web of Science
引用统计	被引频次[WOS]：19
成果类型	期刊论文
条目标识符	http://sustech.caswiz.com/handle/2SGJ60CL/647427
专题	工学院_环境科学与工程学院
作者单位	1.East China Univ Technol, Sch Chem & Mat Sci, Jiangxi Prov Key Lab Synthet Chem, Jiangxi Key Lab Mass Spectrometry & Instrumentat, Nanchang 330013, Peoples R China 2.Southern Univ Sci & Technol, Sch Environm Sci & Engn, Shenzhen 518055, Peoples R China
通讯作者单位	环境科学与工程学院
推荐引用方式 GB/T 7714	Liu, Yu-Feng,Hu, Qi-Long,Chen, Xue-Jiao,et al. Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles[J]. RARE METALS,2023.
APA	Liu, Yu-Feng,Hu, Qi-Long,Chen, Xue-Jiao,Li, Ke,Luo, Pei,&Yang, Guo-Ping.(2023).Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles.RARE METALS.
MLA	Liu, Yu-Feng,et al."Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles".RARE METALS (2023).