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题名

High Sensitivity and Low Detection Limit of Formaldehyde Sensor Based on In2O3@ZnO@ZIF-CoZn Core Shell Nanofibers

作者
发表日期
2024
DOI
发表期刊
ISSN
2379-9153
卷号PP期号:99
摘要
High sensitivity and low detection limit of formaldehyde sensors are extremely essential for indoor air pollution monitoring. Herein, we propose a controllable strategy for the construction of metal oxide semiconductor@metal organic framework (MOS@MOF) core-shell architectures as the sensing material. In2O3@ZnO core-shell nanofibers (IZO CSNFs) are prefabricated by combining electrospinning and atomic layer deposition (ALD) technique, where the ALD-ZnO layer can be regarded as template to obtain cobalt-doped ZIF-8 (ZIF-CoZn) sheath. In comparison to initial IZO CSNFs, the response of IZO@ZIF-CoZn sensor toward 50 ppm formaldehyde can be boosted from 6.6 to 39.4 at 260 °C, and the limit of detection can be as low as 2.1 ppb (@ 20% relative humidity). The enhanced performance of the IZO@ZIF-CoZn sensor should result from the highly efficient adsorption/decomposition of formaldehyde on the surface of ZIF-CoZn. In addition, the effects of core-shell structure, cobalt dopants, interference gases, and moisture on the formaldehyde gas sensing are discussed. Our results provide an insight into the enhancement mechanism of the MOS-based gas sensors by utilizing the functionalized MOF sheaths.
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ESI学科分类
ENGINEERING
引用统计
成果类型期刊论文
条目标识符http://sustech.caswiz.com/handle/2SGJ60CL/783754
专题工学院_深港微电子学院
作者单位
1.Institutes of Physical Science and Information Technology, Anhui University, Hefei, China
2.School of Microelectronics, Southern University of Science and Technology, Shenzhen, China
推荐引用方式
GB/T 7714
Changhui Zhao,Suye Pan,Xiaohui Li,et al. High Sensitivity and Low Detection Limit of Formaldehyde Sensor Based on In2O3@ZnO@ZIF-CoZn Core Shell Nanofibers[J]. IEEE Sensors Journal,2024,PP(99).
APA
Changhui Zhao,Suye Pan,Xiaohui Li,Xi Tang,&Fei Wang.(2024).High Sensitivity and Low Detection Limit of Formaldehyde Sensor Based on In2O3@ZnO@ZIF-CoZn Core Shell Nanofibers.IEEE Sensors Journal,PP(99).
MLA
Changhui Zhao,et al."High Sensitivity and Low Detection Limit of Formaldehyde Sensor Based on In2O3@ZnO@ZIF-CoZn Core Shell Nanofibers".IEEE Sensors Journal PP.99(2024).
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