南方科技大学知识苑(SUSTech KC): Pseudo-nanostructure and trapped-hole release induce high thermoelectric performance in PbTe

题名	Pseudo-nanostructure and trapped-hole release induce high thermoelectric performance in PbTe
作者	Jia, Baohai 1 ; Wu, Di 2; Xie, Lin1 ; Wang, Wu1 ; Yu, Tian 3; Li, Shangyang1 ; Wang, Yan1 ; Xu, Yanjun 4; Jiang, Binbin 5; Chen, Zhiquan 3; Weng, Yuxiang 4; He, Jiaqing1
通讯作者	He, Jiaqing
发表日期	2024-04-05
DOI	10.1126/science.adj8175
发表期刊	SCIENCE 影响因子和分区
ISSN	0036-8075
EISSN	1095-9203
卷号	384 期号:6691
摘要	Thermoelectric materials can realize direct and mutual conversion between electricity and heat. However, developing a strategy to improve high thermoelectric performance is challenging because of strongly entangled electrical and thermal transport properties. We demonstrate a case in which both pseudo-nanostructures of vacancy clusters and dynamic charge-carrier regulation of trapped-hole release have been achieved in p-type lead telluride-based materials, enabling the simultaneous regulations of phonon and charge carrier transports. We realized a peak zT value up to 2.8 at 850 kelvin and an average zT value of 1.65 at 300 to 850 kelvin. We also achieved an energy conversion efficiency of similar to 15.5% at a temperature difference of 554 kelvin in a segmented module. Our demonstration shows promise for mid-temperature thermoelectrics across a range of different applications.
相关链接	[来源记录]
收录类别	SCI
语种	英语
学校署名	第一 ; 通讯
资助项目	National Natural Science Foundation of China[11934007] ; Science and Technology Innovation Committee Foundation of Shenzhen["JCYJ20200109141205978","ZDSYS20141118160434515"] ; Outstanding Talents Training Fund in Shenzhen[202108] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB33000000]
WOS研究方向	Science & Technology - Other Topics
WOS类目	Multidisciplinary Sciences
WOS记录号	WOS:001253335100033
出版者	AMER ASSOC ADVANCEMENT SCIENCE
ESI学科分类	BIOLOGY & BIOCHEMISTRY ; CLINICAL MEDICINE ; MULTIDISCIPLINARY ; PLANT & ANIMAL SCIENCE ; ENVIRONMENT/ECOLOGY ; SOCIAL SCIENCES, GENERAL ; MICROBIOLOGY ; ECONOMICS BUSINESS ; IMMUNOLOGY ; MATERIALS SCIENCE ; MATHEMATICS ; COMPUTER SCIENCE ; SPACE SCIENCE ; MOLECULAR BIOLOGY & GENETICS ; CHEMISTRY ; PSYCHIATRY/PSYCHOLOGY ; NEUROSCIENCE & BEHAVIOR ; PHYSICS ; GEOSCIENCES ; ENGINEERING
来源库	Web of Science
引用统计	被引频次[WOS]：55
成果类型	期刊论文
条目标识符	http://sustech.caswiz.com/handle/2SGJ60CL/787088
专题	理学院_物理系
作者单位	1.Southern Univ Sci & Technol, Dept Phys, Shenzhen Key Lab Thermoelectr Mat, Shenzhen 518055, Peoples R China 2.Shaanxi Normal Univ, Sch Mat Sci & Engn, Key Lab Macromol Sci Shaanxi Prov, Xian 710119, Peoples R China 3.Wuhan Univ, Dept Phys, Hubei Nucl Solid Phys Key Lab, Wuhan 430072, Peoples R China 4.Chinese Acad Sci, Lab Soft Matter Phys, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China 5.Univ Elect Sci & Technol China, Sch Mat & Energy, Chengdu 610054, Peoples R China
第一作者单位	物理系
通讯作者单位	物理系
第一作者的第一单位	物理系
推荐引用方式 GB/T 7714	Jia, Baohai,Wu, Di,Xie, Lin,et al. Pseudo-nanostructure and trapped-hole release induce high thermoelectric performance in PbTe[J]. SCIENCE,2024,384(6691).
APA	Jia, Baohai.,Wu, Di.,Xie, Lin.,Wang, Wu.,Yu, Tian.,...&He, Jiaqing.(2024).Pseudo-nanostructure and trapped-hole release induce high thermoelectric performance in PbTe.SCIENCE,384(6691).
MLA	Jia, Baohai,et al."Pseudo-nanostructure and trapped-hole release induce high thermoelectric performance in PbTe".SCIENCE 384.6691(2024).