南方科技大学知识苑(SUSTech KC): Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase

题名	Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase
作者	Wu, Wei 1; Niu, Fang 1,2; Sun, Chuankui 1,2; Wang, Qingrong3 ; Wang, Man3 ; Wang, Jun3 ; Deng, Yonghong3 ; Ning, De 1; Li, Wenjie 1; Zhang, Jie 1; Chen, Ming 1; Cheng, Hui-Ming 4,5; Yang, Chunlei 1,5
通讯作者	Wu, Wei; Wang, Jun; Cheng, Hui-Ming; Yang, Chunlei
发表日期	2024-06-01
DOI	10.1002/adma.202404630
发表期刊	ADVANCED MATERIALS 影响因子和分区
ISSN	0935-9648
EISSN	1521-4095
摘要	The extreme fast charging performance of lithium metal batteries (LMBs) with a long life is an important focus in the development of next-generation battery technologies. The friable solid electrolyte interphase and dendritic lithium growth are major problems. The formation of an inorganic nanocrystal-dominant interphase produced by preimmersing the Li in molten lithium bis(fluorosulfonyl)imide that suppresses the overgrowth of the usual interphase is reported. Its high surface modulus combined with fast Li+ diffusivity enables a reversible dendrite-proof deposition under ultrahigh-rate conditions. It gives a record-breaking cumulative plating/stripping capacity of >240 000 mAh cm(-2) at 30 mA cm(-2)@30 mAh cm(-2) for a symmetric cell and an extreme fast charging performance at 6 C for 500 cycles for a Li\|\|LiCoO2 full cell with a high-areal-capacity, thus expanding the use of LMBs to high-loading and power-intensive scenarios. Its usability both in roll-to-roll production and in different electrolytes indicating the scalable and industrial potential of this process for high-performance LMBs.
关键词	anode dendrite extreme fast charging lithium metal battery roll-to-roll solid electrolyte interphase
相关链接	[来源记录]
收录类别	SCI ; EI
语种	英语
学校署名	通讯
资助项目	Basic and Applied Basic Research Foundation of Guangdong Province[2022A1515110313] ; Shenzhen Science and Technology Program[JCYJ20230807140818040] ; null[52173243] ; null[52002393] ; null[52202331]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号	WOS:001250156000001
出版者	WILEY-V C H VERLAG GMBH
ESI学科分类	MATERIALS SCIENCE
来源库	Web of Science
引用统计	被引频次[WOS]：4
成果类型	期刊论文
条目标识符	http://sustech.caswiz.com/handle/2SGJ60CL/787818
专题	创新创业学院
作者单位	1.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China 2.Univ Sci & Technol China, Nano Sci & Technol Inst, Suzhou 215123, Peoples R China 3.Southern Univ Sci & Technol, Sch Innovat & Entrepreneurship, Shenzhen 518055, Peoples R China 4.Chinese Acad Sci, Inst Technol Carbon Neutral, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China 5.Shenzhen Univ Adv Technol, Fac Mat Sci & Engn, Shenzhen 518107, Peoples R China
通讯作者单位	创新创业学院
推荐引用方式 GB/T 7714	Wu, Wei,Niu, Fang,Sun, Chuankui,et al. Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase[J]. ADVANCED MATERIALS,2024.
APA	Wu, Wei.,Niu, Fang.,Sun, Chuankui.,Wang, Qingrong.,Wang, Man.,...&Yang, Chunlei.(2024).Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase.ADVANCED MATERIALS.
MLA	Wu, Wei,et al."Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase".ADVANCED MATERIALS (2024).