Advancing high-performance one-dimensional Si/carbon anodes: Current status and challenges

Chen, Xinyu1,2; Mu, Yongbiao1,2; Liao, Zifan1,2; Chu, Youqi1,2; Kang, Shaowei1,2; Wu, Bu-ke1,2; Liao, Ruixi1,2; Han, Meisheng1,2; Li, Yiju1,2; Zeng, Lin1,2

2024-03-01

10.1002/cnl2.118

CARBON NEUTRALIZATION   影响因子和分区

2769-3333

2769-3325

["Silicon (Si) anodes, known for their high capacity, confront obstacles such as volume expansion, the solid-electrolyte interface (SEI) formation, and limited cyclability, driving ongoing research for innovative solutions to enhance their performance in next-generation lithium-ion batteries (LIBs). This comprehensive review explores the forefront of one-dimensional (1D) Si/carbon anodes for high-performance LIBs. This review delves into cutting-edge strategies for fabricating 1D Si/carbon structures, such as nanowires, nanotubes, and nanofibers, highlighting their advantages in mitigating volume expansion, enhancing electron/ion transport, and bolstering cycling stability. The review showcases remarkable achievements in 1D Si/carbon anode performance, including exceptional capacity retention, high-rate capability, and prolonged cycle life. Challenges regarding scalability, cost-effectiveness, and long-term stability are addressed, providing insights into the path to commercialization. Additionally, future directions and potential breakthroughs are outlined, guiding researchers and industries toward harnessing the potential of 1D Si/carbon anodes in revolutionizing energy storage.","Silicon-carbon (Si/C) materials are widely recognized as the next-generation anode materials for lithium-ion batteries due to their high theoretical specific capacity and low-cost advantages. However, severe volume expansion limits its further steps toward the market. The construction of one-dimensional (1D) nanosized silicon-carbon anode materials by structural design is a solution to the problem of swelling. In this review, we systematically introduce the structures, properties, and synthesis processes of different components of 1D Si/C materials by a discrete approach, and address the challenges and development prospects of 1D Si/C materials based on the latest reports. Some constructive suggestions for their commercialization are outlined in the end. image"]

1D Si/carbon high-performance lithium-ion batteries Si anodes Si nanosizing

ESCI

英语

第一 ; 通讯

Stable Support Plan Program for Higher Education Institutions[20220815094504001] ; null[202204013000060]

Science & Technology - Other Topics ; Materials Science

Green & Sustainable Science & Technology ; Materials Science, Multidisciplinary

WOS:001235417500002

WILEY

Web of Science

1.Southern Univ Sci & Technol, Dept Mech & Energy Engn, Shenzhen Key Lab Adv Energy Storage, Shenzhen 518055, Peoples R China
2.Southern Univ Sci & Technol, SUSTech Energy Inst Carbon Neutral, Shenzhen, Peoples R China

Chen, Xinyu,Mu, Yongbiao,Liao, Zifan,et al. Advancing high-performance one-dimensional Si/carbon anodes: Current status and challenges[J]. CARBON NEUTRALIZATION,2024,3(2).

Chen, Xinyu.,Mu, Yongbiao.,Liao, Zifan.,Chu, Youqi.,Kang, Shaowei.,...&Zeng, Lin.(2024).Advancing high-performance one-dimensional Si/carbon anodes: Current status and challenges.CARBON NEUTRALIZATION,3(2).

Chen, Xinyu,et al."Advancing high-performance one-dimensional Si/carbon anodes: Current status and challenges".CARBON NEUTRALIZATION 3.2(2024).