题名 | Photodissociation dynamics of SO2 via the G1B1 state: The O(1D2) and O(1S0) product channels |
作者 | |
通讯作者 | Chang, Yao; Yu, Shengrui; Yuan, Kaijun |
发表日期 | 2024-04-28
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DOI | |
发表期刊 | |
ISSN | 0021-9606
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EISSN | 1089-7690
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卷号 | 160期号:16 |
摘要 | Produced by both nature and human activities, sulfur dioxide (SO2) is an important species in the earth's atmosphere. SO2 has also been found in the atmospheres of other planets and satellites in the solar system. The photoabsorption cross sections and photodissociation of SO2 have been studied for several decades. In this paper, we reported the experimental results for photodissociation dynamics of SO2 via the G1B1 state. By analyzing the images from the time-sliced velocity map ion imaging method, the vibrational state population distributions and anisotropy parameters were obtained for the O(1D2) + SO(X3 Sigma-, a1 Delta, b1 Sigma+) and O(1S0) + SO(X3 Sigma-) channels, and the branching ratios for the channels O(1D2) + SO(X3 Sigma-), O(1D2) + SO(a1 Delta), and O(1D2) + SO(b1 Sigma+) were determined to be similar to 0.3, similar to 0.6, and similar to 0.1, respectively. The SO products were dominant in electronically and rovibrationally excited states, which may have yet unrecognized roles in the upper planetary atmosphere. |
相关链接 | [来源记录] |
收录类别 | |
语种 | 英语
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学校署名 | 其他
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资助项目 | the National Natural Science Foundation of China[22288201]
; National Natural Science Foundation of China[GJJSTD20220001]
; Scientific Instrument Developing Project of the Chinese Academy of Sciences[2021ZD0303304]
; Innovation Program for Quantum Science and Technology["2019ZT08L455","2019JC01X091"]
; Guangdong Science and Technology Program[ZDSYS20200421111001787]
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WOS研究方向 | Chemistry
; Physics
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WOS类目 | Chemistry, Physical
; Physics, Atomic, Molecular & Chemical
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WOS记录号 | WOS:001208022000011
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出版者 | |
ESI学科分类 | CHEMISTRY
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来源库 | Web of Science
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引用统计 | |
成果类型 | 期刊论文 |
条目标识符 | http://sustech.caswiz.com/handle/2SGJ60CL/788569 |
专题 | 理学院_化学系 南方科技大学 |
作者单位 | 1.Chinese Acad Sci, State Key Lab Mol React Dynam, Dalian Coherent Light Source & Dalian Inst Chem Ph, 457 Zhongshan Rd, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Zhejiang Normal Univ, Hangzhou Inst Adv Studies, 1108 Gengwen Rd, Hangzhou 311231, Zhejiang, Peoples R China 4.Hefei Natl Lab, Hefei 230088, Peoples R China 5.Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China 6.Southern Univ Sci & Technol, Coll Sci, Ctr Adv Light Source Res, Shenzhen 518055, Peoples R China |
推荐引用方式 GB/T 7714 |
Wu, Yucheng,Sun, Jitao,Li, Zhenxing,et al. Photodissociation dynamics of SO2 via the G1B1 state: The O(1D2) and O(1S0) product channels[J]. JOURNAL OF CHEMICAL PHYSICS,2024,160(16).
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APA |
Wu, Yucheng.,Sun, Jitao.,Li, Zhenxing.,Zhang, Zhaoxue.,Luo, Zijie.,...&Yang, Xueming.(2024).Photodissociation dynamics of SO2 via the G1B1 state: The O(1D2) and O(1S0) product channels.JOURNAL OF CHEMICAL PHYSICS,160(16).
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MLA |
Wu, Yucheng,et al."Photodissociation dynamics of SO2 via the G1B1 state: The O(1D2) and O(1S0) product channels".JOURNAL OF CHEMICAL PHYSICS 160.16(2024).
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