Bottom-Up Film-to-Bulk Assembly Toward Bioinspired Bulk Structural Nanocomposites

Chen, Si-Ming1; Zhang, Zhen-Bang2; Gao, Huai-Ling1,3; Yu, Shu-Hong1,2

2024-06-01

10.1002/adma.202313443

ADVANCED MATERIALS   影响因子和分区

0935-9648

1521-4095

["Biological materials, although composed of meager minerals and biopolymers, often exhibit amazing mechanical properties far beyond their components due to hierarchically ordered structures. Understanding their structure-properties relationships and replicating them into artificial materials would boost the development of bulk structural nanocomposites. Layered microstructure widely exists in biological materials, serving as the fundamental structure in nanosheet-based nacres and nanofiber-based Bouligand tissues, and implying superior mechanical properties. High-efficient and scalable fabrication of bioinspired bulk structural nanocomposites with precise layered microstructure is therefore important yet remains difficult. Here, one straightforward bottom-up film-to-bulk assembly strategy is focused for fabricating bioinspired layered bulk structural nanocomposites. The bottom-up assembly strategy inherently offers a methodology for precise construction of bioinspired layered microstructure in bulk form, availability for fabrication of bioinspired bulk structural nanocomposites with large sizes and complex shapes, possibility for design of multiscale interfaces, feasibility for manipulation of diverse heterogeneities. Not limited to discussing what has been achieved by using the current bottom-up film-to-bulk assembly strategy, it is also envisioned how to promote such an assembly strategy to better benefit the development of bioinspired bulk structural nanocomposites. Compared to other assembly strategies, the highlighted strategy provides great opportunities for creating bioinspired bulk structural nanocomposites on demand.","Bioinspired bulk structural nanocomposites have received extensive attention owing to the requirements of structural applications. In this review, the bottom-up film-to-bulk assembly strategy is highlighted as a simple, flexible, and scalable path toward fabricating bioinspired bulk structural nanocomposites on demand. Specifically, its design principles, comprehensive advantages, flexible extensions, along with recent advances in bioinspired structural materials are discussed, respectively. image"]

bionics bottom-up film-to-bulk assembly bulk structural nanocomposites layered structure mechanical properties

SCI ; EI

英语

通讯

National Natural Science Foundation of China["22293044","22005289","92263102"] ; Major Basic Research Project of Anhui Province[2023z04020009] ; USTC Research Funds of the Double First-Class Initiative[YD9990002019] ; null[2021YFA0715700] ; null[2018YFE0202201]

Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics

Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter

WOS:001181551200001

WILEY-V C H VERLAG GMBH

MATERIALS SCIENCE

Web of Science

1.Univ Sci & Technol China, Hefei Natl Res Ctr Phys Sci Microscale, Inst Biomimet Mat & Chem, Anhui Engn Lab Biomimet Mat,Dept Chem,Div Nanomat, Hefei 230026, Peoples R China
2.Southern Univ Sci & Technol, Inst Innovat Mat, Guangming Adv Res Inst, Dept Mat Sci & Engn,Dept Chem,Shenzhen Key Lab Sus, Shenzhen 518055, Peoples R China
3.Univ Sci & Technol China, Dept Modern Mech, CAS Key Lab Mech Behav & Design Mat, Hefei 230027, Peoples R China

Chen, Si-Ming,Zhang, Zhen-Bang,Gao, Huai-Ling,et al. Bottom-Up Film-to-Bulk Assembly Toward Bioinspired Bulk Structural Nanocomposites[J]. ADVANCED MATERIALS,2024,36(23).

Chen, Si-Ming,Zhang, Zhen-Bang,Gao, Huai-Ling,&Yu, Shu-Hong.(2024).Bottom-Up Film-to-Bulk Assembly Toward Bioinspired Bulk Structural Nanocomposites.ADVANCED MATERIALS,36(23).

Chen, Si-Ming,et al."Bottom-Up Film-to-Bulk Assembly Toward Bioinspired Bulk Structural Nanocomposites".ADVANCED MATERIALS 36.23(2024).