Photo-steered rapid and multimodal locomotion of 3D-printed tough hydrogel robots

Dong, Min1; Liu, Weixuan2; Dai, Chen Fei1; Jiao, Dejin1; Zhu, Qing Li1; Hong, Wei2; Yin, Jun3; Zheng, Qiang1; Wu, Zi Liang1

2024-05-07

10.1039/d3mh02247a

MATERIALS HORIZONS   影响因子和分区

2051-6347

2051-6355

["Hydrogels are an ideal material to develop soft robots. However, it remains a grand challenge to develop miniaturized hydrogel robots with mechanical robustness, rapid actuation, and multi-gait motions. Reported here is a facile strategy to fabricate hydrogel-based soft robots by three-dimensional (3D) printing of responsive and nonresponsive tough gels for programmed morphing and locomotion upon stimulations. Highly viscoelastic poly(acrylic acid-co-acrylamide) and poly(acrylic acid-co-N-isopropyl acrylamide) aqueous solutions, as well as their mixtures, are printed with multiple nozzles into 3D constructs followed by incubation in a solution of zirconium ions to form robust carboxyl-Zr4+ coordination complexes, to produce tough metallo-supramolecular hydrogel fibers. Gold nanorods are incorporated into ink to afford printed gels with response to light. Owing to the mechanical excellence and small diameter of gel fibers, the printed hydrogel robots exhibit high robustness, fast response, and agile motions when remotely steered by dynamic light. The design of printed constructs and steering with spatiotemporal light allow for multimodal motions with programmable trajectories of the gel robots. The hydrogel robots can walk, turn, flip, and transport cargos upon light stimulations. Such printed hydrogels with good mechanical performances, fast response, and agile locomotion may open opportunities for soft robots in biomedical and engineering fields.","Tough hydrogel-based soft robots are devised by extrusion-based 3D printing of metallosupramolecular gels with different responses, which exhibit agile multi-gait locomotion and task execution upon dynamic light stimulations."]

SCI ; EI

英语

其他

National Natural Science Foundation of China["52325302","51973189","52173012","2022SZ-FR004"]

Chemistry ; Materials Science

Chemistry, Multidisciplinary ; Materials Science, Multidisciplinary

WOS:001166392400001

ROYAL SOC CHEMISTRY

Web of Science

1.Zhejiang Univ, Dept Polymer Sci & Engn, Minist Educ, Key Lab Macromol Synth & Functionalizat, Hangzhou 310058, Peoples R China
2.Southern Univ Sci & Technol, Dept Mech & Aerosp Engn, Shenzhen Key Lab Soft Mech & Smart Mfg, Shenzhen 518055, Peoples R China
3.Zhejiang Univ, Sch Mech Engn, State Key Lab Fluid Power & Mechatron Syst, Key Lab 3D Printing Proc & Equipment Zhejiang Prov, Hangzhou 310027, Peoples R China

Dong, Min,Liu, Weixuan,Dai, Chen Fei,et al. Photo-steered rapid and multimodal locomotion of 3D-printed tough hydrogel robots[J]. MATERIALS HORIZONS,2024,11(9).

Dong, Min.,Liu, Weixuan.,Dai, Chen Fei.,Jiao, Dejin.,Zhu, Qing Li.,...&Wu, Zi Liang.(2024).Photo-steered rapid and multimodal locomotion of 3D-printed tough hydrogel robots.MATERIALS HORIZONS,11(9).

Dong, Min,et al."Photo-steered rapid and multimodal locomotion of 3D-printed tough hydrogel robots".MATERIALS HORIZONS 11.9(2024).